Steve Rogers / Captain America
Natasha Romanoff / Black Widow
Bucky Barnes / Winter Soldier
Maximiliano Hernandez
Jasper Sitwell
Emily VanCamp
Kate / Agent 13
Stan Lee
Smithsonian Guard
Callan Mulvey
Jack Rollins
Bernard White
Councilman Singh
Alan Dale
Councilman Rockwell
Georges St-Pierre
Georges Batroc
Salvator Xuereb
French Pirate #1
Brian Duffy
French Pirate #2
Adetokumboh MCormack
French Radio Pirate
Christopher George Sarris
Skinny Steve
Aaron Himelstein
Launch Tech #1
Allan Chanes
Launch Tech #2
Christopher Markus
SHIELD Interrogator #1
Stephen McFeely
SHIELD Interrogator #2
D.C. Pierson
Apple Employee
Angela Russo-Otstot
Garcia
Chad Todhunter
Charlie Weapons Tech
Abigail Marlowe
SHIELD Tech
Jeremy Maxwell
Lead SHIELD Pilot
Emerson Brooks
Senior SHIELD Agent
Ricardo Chacon
Strike SGT. #1
Michael Debeljak
Strike Agent
Eddie J. Fernandez
Strike Agent
Jody Hart
25ᵗʰ Floor Strike Agent
Derek Hughes
Human Resources Executive
Dominic Rains
CIA Instructor
Charles Wittman
Capitol Hill Police
Terence O'Rourke
FBI Agent
Anne Grimenstein
Committee Member
Dante Rosalina
Little Boy in the Smithsonian
Robert Clotworthy
Fury Car Voice (voice)
June Christopher
SHIELD Computer (voice)
Gary Sinise
The Smithsonian Narrator (voice)
Dean Barlage
SHIELD Agent (uncredited)
Henry Goodman
Dr. List (uncredited)
Josh Heileman
S.H.I.E.L.D. Strike Agent (uncredited)
Dominique Henderson
Pedestrian (uncredited)
Thomas Kretschmann
Baron Wolfgang von Strucker (uncredited)
James Lewis
Smithsonian Museum Visitor
Wanda Maximoff / Scarlet Witch (uncredited)
Nestor Serrano
Committee General (uncredited)
Pietro Maximoff / Quicksilver (uncredited)
Joel Thingvall
Museum Visitor (uncredited)